For solid–liquid mixtures, the reactive uptake coefficient depended on exposure time: the uptake decreased by a factor of 10 after exposure to NO3 for approximately 90 min. V chem shodstvo drevnegrecheskogo i drevnerimskogo teatrov. These studies were carried out to better understand the reactivity of unsaturated organics in multicomponent and multiphase atmospheric particles. Bertram* Received 27th November 2010, Accepted 3rd February 2011 DOI: 10.1039/c0cp02682d We investigated the reactive uptake of NO3 (an important night-time oxidant in the atmosphere) on binary mixtures containing an unsaturated organic (methyl oleate) and saturated molecules (diethyl sebacate, dioctyl sebacate, and squalane) which we call matrix molecules. For liquid binary mixtures the reactivity of methyl oleate depended on the matrix molecule. Assuming a bulk reaction, Hmatrix ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi Dmatrixkoleate p varied by a factor of 2.7, and assuming a surface reaction HSmatrixK S matrixk S oleate varied by a factor of 3.6, where Hmatrix ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi Dmatrixkoleate p and HSmatrixK S matrixk S oleate are constants extracted from the data using the resistor model.

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